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The electrochemistry and spectroelectrochemistry of Ru(porphyrin)(NO)(phenoxide) complexes indicate that initial one-electron oxidation results in structure-dependent net reactivity at the phenoxide ligand. 

Many discriminative natural language understanding (NLU) tasks have large label spaces. Learning such a process of large-space decision making is particularly challenging due to the lack of training instances per label and the difficulty of selection among many fine-grained labels. Inspired by dense retrieval methods for passage finding in open-domain QA, we propose a reformulation of large-space discriminative NLU tasks as a learning-to-retrieve task, leading to a novel solution named Dense Decision Retrieval (DDR). Instead of predicting fine-grained decisions as logits, DDR adopts a dual-encoder architecture that learns to predict by retrieving from a decision thesaurus. This approach not only leverages rich indirect supervision signals from easy-to-consume learning resources for dense retrieval, it also leads to enhanced prediction generalizability with a semantically meaningful representation of the large decision space. When evaluated on tasks with decision spaces ranging from hundreds to hundred-thousand scales, DDR outperforms strong baselines greatly by 27.54% in P @1 on two extreme multi-label classification tasks, 1.17% in F1 score ultra-fine entity typing, and 1.26% in accuracy on three few-shot intent classification tasks on average. 

Entity typing aims at predicting one or more words that describe the type(s) of a specific mention in a sentence. Due to shortcuts from surface patterns to annotated entity labels and biased training, existing entity typing models are subject to the problem of spurious correlations. To comprehensively investigate the faithfulness and reliability of entity typing methods, we first systematically define distinct kinds of model biases that are reflected mainly from spurious correlations. Particularly, we identify six types of existing model biases, including mention-context bias, lexical overlapping bias, named entity bias, pronoun bias, dependency bias, and overgeneralization bias. To mitigate model biases, we then introduce a counterfactual data augmentation method. By augmenting the original training set with their debiasedcounterparts, models are forced to fully comprehend sentences and discover the fundamental cues for entity typing, rather than relying on spurious correlations for shortcuts. Experimental results on the UFET dataset show our counterfactual data augmentation approach helps improve generalization of different entity typing models with consistently better performance on both the original and debiased test sets.